Jose Mourinho has now won the League Cup four times, a joint-record among managers along with Brian Clough and former Manchester United boss Sir Alex Ferguson.
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United played out a thrilling Wembley final with Southampton on Sunday, with Zlatan Ibrahimovic scoring twice to secure the trophy for the Red Devils.
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Manolo Gabbiadini had an early goal ruled out for offside but went on to score twice, levelling the game after Jesse Lingard put United 2-0 up in the first half.
Ibrahimovic struck three minutes from time, though, securing United’s fifth League Cup trophy, and Mourinho’s fourth.
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The Portuguese led Chelsea to the trophy in 2005, 2007 and 2015, with Sunday’s victory his first major trophy as United boss.
Mourinho also became the first manager to win a major trophy in his first season at Old Trafford.